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dc.contributor.authorBatmunkh, M.en
dc.contributor.authorShrestha, A.en
dc.contributor.authorBat-Erdene, M.en
dc.contributor.authorNine, M.en
dc.contributor.authorShearer, C.en
dc.contributor.authorGibson, C.en
dc.contributor.authorSlattery, A.en
dc.contributor.authorTawfik, S.en
dc.contributor.authorFord, M.en
dc.contributor.authorDai, S.en
dc.contributor.authorQiao, S.en
dc.contributor.authorShapter, J.en
dc.identifier.citationAngewandte Chemie International Edition, 2018; 57(10):2644-2647en
dc.description.abstractResearch into efficient synthesis, fundamental properties, and potential applications of phosphorene is currently the subject of intense investigation. Herein, solution-processed phosphorene or few-layer black phosphorus (FL-BP) sheets are prepared using a microwave exfoliation method and used in photoelectrochemical cells. Based on experimental and theoretical (DFT) studies, the FL-BP sheets are found to act as catalytically active sites and show excellent electrocatalytic activity for triiodide reduction in dye-sensitized solar cells. Importantly, the device fabricated based on the newly designed cobalt sulfide (CoSx ) decorated nitrogen and sulfur co-doped carbon nanotube heteroelectrocatalyst coated with FL-BP (FL-BP@N,S-doped CNTs-CoSx ) displayed an impressive photovoltaic efficiency of 8.31 %, outperforming expensive platinum based cells. This work paves the way for using phosphorene-based electrocatalysts for next-generation energy-storage systems.en
dc.description.statementofresponsibilityMunkhbayar Batmunkh, Aabhash Shrestha, Munkhjargal Bat-Erdene, Md Julker Nine, Cameron J. Shearer, Christopher T. Gibson, Ashley D. Slattery, Sherif Abdulkader Tawfik, Michael J. Ford, Sheng Dai, Shizhang Qiao, and Joseph G. Shapteren
dc.rights© 2018 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheimen
dc.subject2D materials; black phosphorus; electrocatalysis; photochemistry; solar cellsen
dc.titleElectrocatalytic activity of a 2D phosphorene-based heteroelectrocatalyst for photoelectrochemical cellsen
dc.typeJournal articleen
pubs.library.collectionChemical Engineering publicationsen
dc.identifier.orcidNine, M. [0000-0002-5740-8627]en
dc.identifier.orcidShearer, C. [0000-0002-8192-3696]en
dc.identifier.orcidSlattery, A. [0000-0003-4023-3506]en
dc.identifier.orcidQiao, S. [0000-0002-1220-1761]en
Appears in Collections:Chemical Engineering publications

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