Please use this identifier to cite or link to this item: https://hdl.handle.net/2440/114452
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dc.contributor.authorTian, W.-
dc.contributor.authorZhang, H.-
dc.contributor.authorSun, H.-
dc.contributor.authorTadé, M.O.-
dc.contributor.authorWang, S.-
dc.date.issued2017-
dc.identifier.citationCarbon, 2017; 118:98-105-
dc.identifier.issn0008-6223-
dc.identifier.issn1873-3891-
dc.identifier.urihttp://hdl.handle.net/2440/114452-
dc.descriptionAvailable online 11 March 2017-
dc.description.abstractCross-linked, N-doped, pillared-layered porous carbons (NCs) were prepared via a one-pot, template-free pyrolysis process at 600 (NC600), 700 (NC700) and 800 °C (NC800), which have bifunctional applications in supercapacitors and environmental remediation. NC700 displays a high surface area (2118 m2 g−1) and a specific capacitance of 305 F g−1 at 0.2 A g−1 in a two-electrode setup. The maximum energy density of NC700 was 20.4 W h/kg at a power density of 139 W kg−1 and 89.1% capacitance was retained after 10000 cycles of charge-discharge at 5 A g−1. For water remediation, NC800 displayed high adsorption capacities towards flame retardant tetrabromobisphenol A (TBBPA, 372 mg g−1) and antibiotic sulfachloropyridazine (SCP, 288 mg g−1) solutions, while NC700 showed the most efficient SCP oxidation removal. These results suggest low-cost and green carbon materials as electrodes in flexible energy storage devices, metal-free adsorbents as well as catalysts for high efficient removal of emerging contaminants in aqueous solution.-
dc.description.statementofresponsibilityWenjie Tian, Huayang Zhang, Hongqi Sun, Moses O.Tadé, Shaobin Wang-
dc.language.isoen-
dc.publisherElsevier-
dc.rights© 2017 Elsevier Ltd. All rights reserved.-
dc.source.urihttp://dx.doi.org/10.1016/j.carbon.2017.03.027-
dc.subjectPorous carbon; supercapacitor; adsorption; advanced oxidation process-
dc.titleTemplate-free synthesis of N-doped carbon with pillared-layered pores as bifunctional materials for supercapacitor and environmental applications-
dc.typeJournal article-
dc.identifier.doi10.1016/j.carbon.2017.03.027-
dc.relation.granthttp://purl.org/au-research/grants/arc/DP130101319-
dc.relation.granthttp://purl.org/au-research/grants/arc/DP150103026-
pubs.publication-statusPublished-
dc.identifier.orcidTian, W. [0000-0002-9896-1154]-
dc.identifier.orcidWang, S. [0000-0002-1751-9162]-
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Chemical Engineering publications

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