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https://hdl.handle.net/2440/134734
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dc.contributor.author | Shang, Y. | - |
dc.contributor.author | Duan, X. | - |
dc.contributor.author | Wang, S. | - |
dc.contributor.author | Yue, Q. | - |
dc.contributor.author | Gao, B. | - |
dc.contributor.author | Xu, X. | - |
dc.date.issued | 2022 | - |
dc.identifier.citation | Chinese Chemical Letters, 2022; 33(2):663-673 | - |
dc.identifier.issn | 1001-8417 | - |
dc.identifier.issn | 1878-5964 | - |
dc.identifier.uri | https://hdl.handle.net/2440/134734 | - |
dc.description.abstract | Carbon-based single-atom catalysts (SACs) with atomic sizes of active sites have become the promising candidates for a variety of catalytic systems because of their high atom utilization, and unique electronic structures. Different types of single-atom sites can be fabricated via multiple preparation strategies, which would demonstrate distinct different coordination configurations and electronic features, and ultimately affected the structure-catalysis relationship of SACs in targeted reactions. As a result, it is necessary to identify the active sites of SACs and understand the structure-catalysis relationship of SACs at the atomic scale. In this review, a variety of preparation strategies of carbon-based SACs were documented. Then, the recent development on versatile characterization techniques and computational achievements were summarized regarding in understanding the electronic and geometric characteristics of carbon-based SACs. Finally, major challenges and development directions concerning single-atom sites identification and advanced tools development are discussed to shed light on future research of carbon-based SACs. | - |
dc.description.statementofresponsibility | Yanan Shang, Xiaoguang Duan, Shaobin Wang, Qinyan Yue, Baoyu Gao, Xing Xu | - |
dc.language.iso | en | - |
dc.publisher | Elsevier | - |
dc.rights | © 2021 Published by Elsevier B.V. on behalf of Chinese Chemical Society and Institute of Materia Medica, Chinese Academy of Medical Sciences. | - |
dc.source.uri | http://dx.doi.org/10.1016/j.cclet.2021.07.050 | - |
dc.subject | Single atom; Synthesis; DFT calculations; Characterization; Catalysis | - |
dc.title | Carbon-based single atom catalyst: Synthesis, characterization, DFT calculations | - |
dc.type | Journal article | - |
dc.identifier.doi | 10.1016/j.cclet.2021.07.050 | - |
dc.relation.grant | http://purl.org/au-research/grants/arc/DE210100253 | - |
pubs.publication-status | Published | - |
dc.identifier.orcid | Duan, X. [0000-0001-9635-5807] | - |
dc.identifier.orcid | Wang, S. [0000-0002-1751-9162] | - |
Appears in Collections: | Chemical Engineering publications |
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