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https://hdl.handle.net/2440/135736
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dc.contributor.author | Ye, H. | - |
dc.contributor.author | Wang, S. | - |
dc.contributor.author | Wang, Y. | - |
dc.contributor.author | Guo, P. | - |
dc.contributor.author | Wang, L. | - |
dc.contributor.author | Zhao, C. | - |
dc.contributor.author | Chen, S. | - |
dc.contributor.author | Chen, Y. | - |
dc.contributor.author | Sun, H. | - |
dc.contributor.author | Wang, S. | - |
dc.contributor.author | Ma, X. | - |
dc.date.issued | 2022 | - |
dc.identifier.citation | Applied Catalysis B: Environmental, 2022; 314:121484-1-121484-11 | - |
dc.identifier.issn | 0926-3373 | - |
dc.identifier.issn | 1873-3883 | - |
dc.identifier.uri | https://hdl.handle.net/2440/135736 | - |
dc.description.abstract | Wastewater remediation using micro/nanomotors is a hot topic, and MnO2 based materials have become fascinating alternatives to rare noble metal-based micro/nanomotors. Herein, we demonstrate facile and large- scale synthesis of Fe-MnO2 core-shell micromotors for antibiotic pollutant removal. Heat-treatment results in a phase transformation of MnO2 with formation of iron oxides and partially exfoliates the MnO2 nanoplate shell structure to promote mobility. The iron-manganese oxide micromotors exhibit an efficient removal of tetracy- cline antibiotics via a combination of catalytic degradation and adsorptive bubble separation. For the first time, atomic H* was found to participate in the micromotor-assisted degradation process, resulting in optimal Fenton reaction in neutral conditions with a good decontamination performance. Owing to the merits of abundance, magnetic recovery, facile fabrication, good motion, and environmental friendliness, as well as decontamination performance in a wide pH range, these core-shell micromotors demonstrate a promising candidate in practical wastewater treatment. | - |
dc.description.statementofresponsibility | Heng Ye, Shengnan Wang, Yong Wang, Peiting Guo, Liying Wang, Chengke Zhao, Shuqing Chen, Yimai Chen, Hongqi Sun, Shaobin Wang, Xing Ma | - |
dc.language.iso | en | - |
dc.publisher | Elsevier BV | - |
dc.rights | © 2022 Elsevier B.V. All rights reserved. | - |
dc.source.uri | http://dx.doi.org/10.1016/j.apcatb.2022.121484 | - |
dc.subject | MnO2 micromotors; Fenton reaction; Catalytic degradation; Adsorptive bubbles separation; Antibiotic removal | - |
dc.title | Atomic H* mediated fast decontamination of antibiotics by bubble-propelled magnetic iron-manganese oxides core-shell micromotors | - |
dc.type | Journal article | - |
dc.identifier.doi | 10.1016/j.apcatb.2022.121484 | - |
dc.relation.grant | http://purl.org/au-research/grants/arc/DP190103548 | - |
pubs.publication-status | Published | - |
dc.identifier.orcid | Wang, S. [0000-0002-1751-9162] | - |
Appears in Collections: | Chemical Engineering publications |
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